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Kesavapillai Sreenath

Florida State University · US
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Area of research
Materials Chemistry · Spectroscopy
Research interest
Research topics from publications: Zn(ii)-coordination modulated ligand photophysical processes – the development of fluorescent indicators for imaging biological Zn(ii) ions; Structurally Diverse Copper(II) Complexes of Polyaza Ligands Containing 1,2,3-Triazoles: Site Selectivity and Magnetic Properties; A Fluorescent Indicator for Imaging Lysosomal Zinc(II) with Förster Resonance Energy Transfer (FRET)‐Enhanced Photostability and a Narrow Band of Emission; Tricolor Emission of a Fluorescent Heteroditopic Ligand over a Concentration Gradient of Zinc(II) Ions; Synthesis of 5-Iodo-1,2,3-triazoles from Organic Azides and Terminal Alkynes: Ligand Acceleration Effect, Substrate Scope, and Mechanistic Insights; Excitation-Dependent Multiple Fluorescence of a Substituted 2-(2′-Hydroxyphenyl)benzoxazole; Absorption and Emission Sensitivity of 2‐(2′‐Hydroxyphenyl)benzoxazole to Solvents and Impurities; Dual Role of Acetate in Copper(II) Acetate Catalyzed Dehydrogenation of Chelating Aromatic Secondary Amines: A Kinetic Case Study of Copper‐Catalyzed Oxidation Reactions; Distinguishing Förster resonance energy transfer and solvent-mediated charge-transfer relaxation dynamics in a zinc(ii) indicator: a femtosecond time-resolved transient absorption spectroscopic study; ChemInform Abstract: Synthesis of 5‐Iodo‐1,2,3‐triazoles from Organic Azides and Terminal Alkynes: Ligand Acceleration Effect, Substrate Scope, and Mechanistic Insights. Representative work: Molecular photophysics and metal coordination chemistry are the two fundamental pillars that support the development of fluorescent cation indicators. In this article, we describe how Zn(II)-coordination alters various ligand-centered photophysical processes that are pertinent to developing Zn(II) indicators. The main aim is to show how small organic Zn(II) indicators work under the constraints of specific requirements, including Zn(II) detection range, photophysical requirements such as excitation energy and emission color, temporal and spatial resolutions in a heterogeneous intracellular environment, and fluorescence response selectivity between similar cations such as Zn(II) and Cd(II). I Copper(II) acetate mediated coupling reactions between 2,6-bis(azidomethyl)pyridine or 2-picolylazide and two terminal alkynes afford 1,2,3-triazolyl-containing ligands L1–L6. These ligands contain various nitrogen-based Lewis b
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Recent publications

Excitation-Dependent Multiple Fluorescence of a Substituted 2-(2′-Hydroxyphenyl)benzoxazole
The Journal of Physical Chemistry A 2018cited by 35position: middledoi
Dual Role of Acetate in Copper(II) Acetate Catalyzed Dehydrogenation of Chelating Aromatic Secondary Amines: A Kinetic Case Study of Copper‐Catalyzed Oxidation Reactions
European Journal of Inorganic Chemistry 2016cited by 22position: firstdoi
Zn(<scp>ii</scp>)-coordination modulated ligand photophysical processes – the development of fluorescent indicators for imaging biological Zn(<scp>ii</scp>) ions
RSC Advances 2014cited by 107position: lastdoi
A Fluorescent Indicator for Imaging Lysosomal Zinc(II) with Förster Resonance Energy Transfer (FRET)‐Enhanced Photostability and a Narrow Band of Emission
Chemistry - A European Journal 2014cited by 52position: firstdoi
Absorption and Emission Sensitivity of 2‐(2′‐Hydroxyphenyl)benzoxazole to Solvents and Impurities
Photochemistry and Photobiology 2014cited by 28position: middledoi
Distinguishing Förster resonance energy transfer and solvent-mediated charge-transfer relaxation dynamics in a zinc(<scp>ii</scp>) indicator: a femtosecond time-resolved transient absorption spectroscopic study
Physical Chemistry Chemical Physics 2014cited by 8position: firstdoi
ChemInform Abstract: Synthesis of 5‐Iodo‐1,2,3‐triazoles from Organic Azides and Terminal Alkynes: Ligand Acceleration Effect, Substrate Scope, and Mechanistic Insights.
ChemInform 2014cited by 0position: middledoi
Synthesis of 5-Iodo-1,2,3-triazoles from Organic Azides and Terminal Alkynes: Ligand Acceleration Effect, Substrate Scope, and Mechanistic Insights
Synthesis 2013cited by 43position: middledoi
Structurally Diverse Copper(II) Complexes of Polyaza Ligands Containing 1,2,3-Triazoles: Site Selectivity and Magnetic Properties
Inorganic Chemistry 2012cited by 89position: middledoi
Tricolor Emission of a Fluorescent Heteroditopic Ligand over a Concentration Gradient of Zinc(II) Ions
The Journal of Organic Chemistry 2012cited by 52position: firstdoi

Grants

No grants ingested yet.

Frequent collaborators

Lei Zhu · Anhui Medical University10 papers (2012–2018)J. Tyler Simmons · Florida State University5 papers (2012–2014)Ronald J. Clark · Florida State University3 papers (2012–2016)Ali H. Younes · Florida State University2 papers (2014–2018)Najeah Okashah · Florida State University2 papers (2013–2014)Christopher J. Brassard · Florida State University2 papers (2013–2014)Jason Deeb · Florida State University2 papers (2013–2014)David N. Barsoum · Florida State University2 papers (2013–2014)Zhenxing Wang · Nanjing Agricultural University1 papers (2012–2012)John R. Allen · Florida State University1 papers (2014–2014)Miguel Macias‐Contreras · Florida State University1 papers (2016–2016)Chongyue Yi · Florida State University1 papers (2014–2014)Joseph J. M. Hurley · Florida State University1 papers (2018–2018)De‐en Jiang · University of California System1 papers (2014–2014)Kenneth L. Knappenberger · Pennsylvania State University1 papers (2014–2014)Naresh S. Dalal · Florida State University1 papers (2012–2012)Qing Tang · University of California System1 papers (2014–2014)Michael Shatruk · Florida State University1 papers (2012–2012)Hoa Phan · National University of Singapore1 papers (2012–2012)Michael W. Davidson · National High Magnetic Field Laboratory1 papers (2014–2014)
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